step 1 - download MSI Afterburner & Kompresor.
step 2 - experiment.
the software is pretty self explanatory. increase clock speeds till it starts crashing one of the kompresor stress tests, then increase power. if it gets hotter then 90C you've probably overclocked it a bit too much (it won't happen, the 7770 is a cool running card, if you get it up over 70C i'll be surprised)