I've heard (don't have an A64 myself) they can do 2.4ghz or so on air pretty easily.
You can bump the fsb up higher by using a memory divider - e.g. set the RAM to 166, then set the fsb to 240 (making the CPU 2.4 at stock multiplier) and your memory is running at 200 - since you have PC3700, at that divider you could run at 276 and not OC your ram (though 2.76ghz on the CPU may be too much - but if you lower the multiplier to 9 that gives you 2.48g).
Also, many ram modules can OC pretty easily with looser timings. I'ts a lot of test change and retest. Read the overclocking sticky at the top of the section for more info on how to do it. You just have to find the max stable setting for each of RAM, FSB & CPU, then find the best mix that gives you the best performance.
Mike.