Thermal Grizzly Hydro is tacky, not thin and oily like Noctua NT-H1. Shouldn't be subject to runoff.
The i7-10750h is direct die, no IHS, so absolutely should always be spatula/cc spread, not pea dropped, you need to guarantee that every single square mm of the die surface is covered. Only use the pea drop if really intending to overload the cpu with a giant pea, not the standard pea. That includes the gpu as well if the heatsink/heatpiping is common to both or was also removed.
One thing to look for is fan rpm. At those temps, the fan should basically be running maxed out. If it's not, that's a good cause of higher than expected temps.
With pump out or runout, the heat/pressure of the heat pipes on straight, glassy silicon will force the paste to squash out from between the heat pipes and the silicon surface. This starts happening immediately, as soon as heat is applied to the paste, and gets gradually worse as what's left thins out to the point of leaving gaps in the surface contact area. But doesn't stop there, it'll continue until you start throttling hard and eventually bsod or shutdown.
So if the temps are back to, and staying in the high 90's, and performance is the same as it was before, and the temps are stable and not continually climbing, I'd say the paste isn't likely the issue, more likely the fan or fan curve or power plan or some other factor.