I would recommend getting a new GPU, as if you went crossfire then the Vram is mirrored, so instead of having 4GB Vram (2x2GB) you get 2GB. The power of dual 270x's seems a bit unbalanced if you only pair it with 2GB of Vram, and therefore you would only double your performance on games that use up to 2GB of Vram. That's just a suggestion, but i'm avid about future proofing my PC, and most likely newer games would require more Vram, so you would require a more powerful card to play them, which then gives you more option to crossfire later.
Hope that helped.
llamington