No, absolutely not. There's no possible way that a gpu can ever bottleneck a cpu.
The cpu pre-renders the frames, as many as it can according to the processor speed, IPC, game code. It then ships those frames to the gpu. The gpu can either have the ability to surpass those frames, or not, depending on detail settings and resolution.
If the cpu sends 100 fps to the gpu, then that's the limit, if the gpu can only put 50fps on screen, that's not slowing the cpu down a bit, the gpu doesn't affect cpu performance at all.
All you've got pairing a gtx750ti with an i5-4670k is a cpu that in most games will not have an issue giving more fps to the gpu than the gpu can put on screen.
Adding a stronger, more powerful gpu will not increase fps...