It's also important to clarify that "not having a bottleneck" doesn't necessarily mean getting "more FPS" though. If you remove the bottleneck by increasing the resolution or quality settings, you are actually likely to end up with FEWER FPS, as it will cause the CPU to not be causing the GPU to wait, hence, no bottleneck, however the GPU will be taking longer to render frames so there will be fewer of them for the CPU to NEED to display, and therefore lower FPS.
The only way to increase FPS, if that is the desire, is by getting a stronger CPU, BUT, that will only increase FPS, IF, the GPU is not now the bottleneck, or, by reducing the quality settings AND having a CPU that can handle the increase in demand for frames.