What are your system specs? And no, you don't have to overclock your RAM to overclock your CPU.
To overclock your CPU you will have to higher the FSB (front side bus) speed. If you higher the FSB speed your CPU clock will get higher because the processor takes the FSB speed and multiplies it by the CPU multiplier.
The same goes for for your memory, higher the FSB then it will be multiplied by the memory multiplier to get your memory frequency.
It's best to start off by lowering memory multiplier and the increasing FSB so that your memory will run at or below its rated speed. Your CPU frequency will rise and then you have to test it for stability using programs such as Prime95. Once you have achieved your overclock goal you can then adjust your memory timings and frequency.
Once you have overclocked you must keep an eye on your temperatures and also run stress tests like Prime95 blend tests which will test your system for stability (excluding GPU's and such).